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Chemical · Seminar 03 · Turning CO₂ back into useful molecules

Electrochemical CO₂ Reduction to Fuels

Electrochemical CO₂ reduction uses renewable electricity to convert captured CO₂ into fuels and chemicals such as CO, formate, ethylene and ethanol, closing the carbon loop.

CO2 reductionelectrocatalysispower-to-Xethyleneselectivity

If we can capture CO₂, the next prize is to use it. Electrochemical CO₂ reduction (CO₂RR) uses renewable electricity to convert CO₂ into valuable products — carbon monoxide, formate, ethylene, ethanol and more — effectively running combustion in reverse and storing clean energy in chemical bonds.

Working principle

In an electrolyser, CO₂ is reduced at the cathode while water is oxidised to O₂ at the anode. The catalyst determines the product: silver and gold favour CO, tin favours formate, and notably copper is uniquely able to form multi-carbon products (ethylene, ethanol). The reaction competes with the unwanted hydrogen-evolution reaction, so selectivity (Faradaic efficiency) is the central metric. Gas-diffusion electrodes feed CO₂ as gas to reach industrially relevant current densities.

reduceionsCO₂ inCathode (Cu / Ag catalyst)CO, C₂H₄, ethanol…Ion-exchange membraneAnode O₂ evolutionH₂OCO₂ electroreduction cell with gas-fed cathode
Figure 1. The cathode catalyst dictates which carbon product forms; copper uniquely enables multi-carbon fuels like ethylene and ethanol.
Table 1. Catalysts and their dominant CO₂RR products
CatalystMain productNote
Silver / goldCOHigh selectivity
Tin / bismuthFormateLow cost
CopperC₂H₄, ethanolOnly metal for C–C coupling
H₂ (parasitic)Competing side reaction
Key challengeThe hard part is achieving high selectivity at high current density with long catalyst life — especially for multi-carbon products on copper, where many pathways compete.

Applications

  • Power-to-X: storing renewable energy as synthetic fuels
  • Sustainable production of ethylene and other chemical feedstocks
  • On-site CO production for industry

References & further reading

  1. Nitopi et al., “Progress and Perspectives of Electrochemical CO₂ Reduction on Copper,” Chemical Reviews, 2019.
  2. De Luna et al., “What would it take for renewably powered electrosynthesis to displace petrochemical processes?,” Science, 2019.
  3. Burdyny & Smith, “CO₂ reduction on gas-diffusion electrodes,” Energy & Environmental Science, 2019.